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Visible Light-Promoted Aerobic Oxidation of α-Silyl Styrenes with Alcohols
  • +2
  • Yan Tan,
  • Bo Yang,
  • Jiale Ying,
  • Bing Yu,
  • Zhan Lu
Yan Tan
Zhengzhou University
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Bo Yang
Zhejiang University
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Jiale Ying
Zhejiang University
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Bing Yu
Zhengzhou University
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Zhan Lu
Zhejiang University

Corresponding Author:[email protected]

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Abstract

A mechanistically distinctive visible-light-promoted metal-free aerobic oxidation of alkenyl silanes with alcohols was disclosed to efficiently construct α-alkoxy ketones under mild conditions. The primary, secondary, and tertiary alcohols could be used as reactants. The protocol could be carried out on a gram-scale. The various derivatizations of products could be conducted. Mechanistic studies indicated the reaction was initiated by single-electron oxidation of the alkenyl silanes.
Submitted to Chinese Journal of Chemistry
14 Jun 2024Reviewer(s) Assigned
12 Jul 2024Review(s) Completed, Editorial Evaluation Pending
12 Jul 2024Editorial Decision: Revise Minor
27 Jul 20241st Revision Received
30 Jul 2024Submission Checks Completed
30 Jul 2024Assigned to Editor
30 Jul 2024Review(s) Completed, Editorial Evaluation Pending
30 Jul 2024Editorial Decision: Accept