This Supporting Information includes:Figure S1, S2, S3Supplementary Video Supplementary Video S1: Locomotion of the mobile robot. Supplementary Video S2: Vortex deforming the liquid-liquid interface. Supplementary Video S3: Locomotion of the mobile robot without electrode attached. Supplementary Video S4: Locomotion of the mobile robot with reversed polarity. Supplementary Video S5: Drawing “SIT” by controlling a floating robot with multiple electrodes. Corresponding author Email: [email protected], [email protected]