Scott Mannis

and 3 more

Examination of historical simulations from CMIP6 models shows substantial pre-industrial to present-day changes in ocean heat (ΔH), salinity (ΔS), oxygen (ΔO2), dissolved inorganic carbon (ΔDIC), chlorofluorocarbon-12 (ΔCFC12), and sulfur hexafluoride (ΔSF6). The spatial structure of the changes and the consistency among models differ among tracers: ΔDIC, ΔCFC12, and ΔSF6 all are largest near the surface, are positive throughout the thermocline with weak changes below, and there is good agreement amongst the models. In contrast, the largest ΔH, ΔS, and ΔO2 are not necessarily at the surface, their sign varies within the thermocline, and there are large differences among models. These differences between the two groups of tracers are linked to climate-driven changes in the ocean transport, with this tracer “redistribution” playing a significant role in changes in ΔH, ΔS, and ΔO2 but not the other tracers. Tracer redistribution is prominent in the southern subtropics, in a region where apparent oxygen utilization and ideal age indicate increased ventilation time scales. The tracer changes are linked to a poleward shift of the peak Southern Hemisphere westerly winds, which causes a similar shift of the subtropical gyres, and anomalous upwelling in the subtropics. This wind - tracer connection is also suggested to be a factor in the large model spread in some tracers, as there is also a large model spread in wind trends. A similar multi-tracer analysis of observations could provide insights into the relative role of the addition and redistribution of tracers in the ocean.

Gaige Hunter Kerr

and 5 more

We investigate the relationships among summertime ozone (O3), temperature, and humidity on daily timescales across the Northern Hemisphere using observations and model simulations. Temperature and humidity are significantly positively correlated with O3 across continental regions in the mid-latitudes (~35-60N). Over the oceans, the relationships are consistently negative. For continental regions outside the mid-latitudes, the O3-meteorology correlations are mixed in strength and sign but generally weak. Over some high latitude, low latitude, and marine regions, temperature and humidity are significantly anticorrelated with O3. Daily variations in transport patterns linked to the position and meridional movement of the jet stream drive the relationships among O3, temperature, and humidity. Within the latitudinal range of the jet, there is an increase (decrease) in O3, temperature, and humidity over land with poleward (equatorward) movement of the jet, while over the oceans poleward movement of the jet results in decreases of these fields. Beyond the latitudes where the jet traverses, the meridional movement of the jet stream has variable or negligible effects on surface-level O3, temperature, and humidity. The O3-meteorology relationships are largely the product of the jet-induced changes in the surface-level meridional flow acting on the background meridional O3 gradient. Our results underscore the importance of considering the role of the jet stream and surface-level flow for the O3-meteorology relationships, especially in light of expected changes to these features under climate change.

Laurie Menviel

and 6 more

The Southern Ocean (SO) provides the largest oceanic sink of carbon. Observational datasets highlight decadal-scale changes in SO CO2 uptake, but the processes leading to this decadal-scale variability remain debated. Here, using an eddy-permitting ocean, sea-ice, carbon cycle model, we explore the impact of changes in Southern Hemisphere (SH) westerlies on contemporary (i.e. total), anthropogenic and natural CO2 fluxes using idealised sensitivity experiments as well as an interannually varying forced (IAF) experiment covering the years 1948 to 2007. We find that a strengthening of the SH westerlies reduces the contemporary CO2 uptake by leading to a high southern latitude natural CO2 outgassing. The enhanced SO upwelling and associated increase in Antarctic Bottom Water decrease the carbon content at depth in the SO, and increase the transport of carbon-rich waters to the surface. A poleward shift of the westerlies particularly enhances the CO2 outgassing south of 60S, while inducing an asymmetrical DIC response between high and mid southern latitudes. Changes in the SH westerlies in the 20th century in the IAF experiment lead to decadal-scale variability in both natural and contemporary CO2 fluxes. The ~10% strengthening of the SH westerlies since the 1980s led to a 0.016 GtC/yr^2 decrease in natural CO2 uptake, while the anthropogenic CO2 uptake increased at a similar rate, thus leading to a stagnation of the total SO CO2 uptake. The projected poleward strengthening of the SH westerlies over the coming century will thus reduce the capability of the SO to mitigate the increase in atmospheric CO2.