This paper explores the integration of uncertainty frameworks such as Fuzzy, Neutrosophic, and Plithogenic sets into Large Language Models (LLMs) and Natural Language Processing (NLP). We propose novel models, including Large Uncertain Language Models and Natural Uncertain Language Processing, to enhance linguistic representations and processing capabilities. Furthermore, we extend the theoretical foundation of LLMs and NLP by incorporating Hyperstructures and Superhyperstructures, enabling higher-order generalizations and hierarchical modeling. These advancements provide new perspectives for addressing uncertainty and complexity in language understanding and processing. While the paper focuses on theoretical generalizations, practical validation through computational experiments remains an important direction for future work.